I haven't decided yet! There's the Nodame Cantabile hug scene (already capped, as you pointed out), the Dark Mercury vs. Sailor Moon fight, possibly the ice cream scene from BOF, the flower scene from Full House (if I can remember what episode it takes place in!), and I still want to get a scene from Mighty Princess. And there's another tearjerker from the One Piece anime that I'm thinking of.

Damn. My capping fingers hurt just thinking about all of those picspams!